We thank Ms. Kazuko Hino for analytical assistance in the laboratory. Special thanks are due to Drs. Yuichiro Tanaka and Masatoshi Komiya, for valuable discussion. Also, thanks are extended to shore-based sampling participants for help in our sampling. The helpful reviews by P.A. Meyers and A. Miller improved the quality of this manuscript. This study was financially supported by the Science and Technology Agency of Japan.